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I personally don't like it because it reminds me of the word harlot. I think Harlow would fit in with her peers Harper, Marlowe (which I prefer for the literary nod) and Harley though. I think Harlow Elise is nice. I would use something classic as a middle name but not a filler name either so
Harlow Lillian
Harlow Lucille
Harlow Pearl
or for something a little bit out there how about Harlow Cosette/Colette?