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They have a bit of a different feel, but they still work as sister names. I think that Tabitha and Charlotte would be a better fit if you want them to have the same feel, though.

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Charlotte is more formal and refined, and Talitha is more unusual and almost mysterious sounding. Talitha is a little hard to say, but I still like it.

I think they sound very nice for sisters, even if they are a bit different in style. Talitha is far less common than Charlotte, so it stands out a lot more.

I'd prefer Tabitha and Charlotte.

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I love Charlotte, but Talitha doesn't do it for me.

I wouldn't think to put them together as sibs. Both are very pretty & sweet names but Charlotte is much more common & heard of than Talitha. I would think Talitha's siblings would have more unusual names.
That said there is nothing wrong with this sibset and they do have similar soft feel to them so if you love both names, use them.

I think they are both lovely names. They are a little different maybe for two sisters. I know how you feel. Theodora and Charlotte are two of my favorite names, and I have always wondered if they were complementary or not.